Zoey is ridiculously perfect like it's not fair

She should voice the next Disney princess, seriously.

She has the sexiest speaking voice and the most amazing singing voice... and she's ridiculously gorgeous! I love you Zooey!!

The original of this song is basically a screaming song, too, so for those who say she's screaming: it's a song written for that sort of performance.

Her serious expression delivering this song is perfect for the subject-mood-delivery. The dress is stunning (as she always is), while this song showcased her surprising vocal range/power and displayed her growing performance confidence. Hope this duo stays together for many more years.

Holy damn McNuggets, I knew she could sing, but I didn't know she had those pipes. They should do more Soul music on their upcoming albums.

I would like to hear her sing Bang Bang My Baby Shot Me Down.

I absolutely love her voice, its so pure and beautiful, she hits every note so perfect! And he is harmonizes with her perfectly! They should be on the radio all the time!

amazing... ethereal, weird, unsettling... beautiful singing and playing... love their music, their look... truly original

This is scarily good. Gave me the goose bumps!

Such a powerful performance! It looks like Zooey isn't even trying to sing, her beautiful "shouting" just flows naturally. Wow! Just wow!

I think you really need to appreciate Zooey's voice and Matt's guitar performance to really understand She & Him. LOVE THIS

I wish she sang with this kind of power on their albums! Holy crap!

Blew my freaking mind. Been on a marathon for her singing because I can't get enough of her vintage voice. I love her range!

to all the people saying "she is shouting, not singing" I WANNA SEE YOU SHOUT LIKE THAT THEN lets see how you do it shall we?

Shouting in perfect key interesting She's doing it for effect and her tone is great.

This voice and that guitar, simply incredible. Can't find one think I don't LOVE about this beautiful human being. ZOOEY, WOO HOO

Shes clearly doesn't need auto tune.. amazing

Woah. This is so alternative and jazzy, and it's just so much emotion... Wow.

I did not know she had such a great voice. I know she could sing, but this was absolutely amazing!

If that song doesn't give you a warm, sexy shiver, you're probably dead ...wow. Just wow.

Mark Ruffalo is killing it with his guitar!

Oh she can sing sing

Doesn't have to be perfect to be beautiful. It's the imperfections that maybe are supposed to be sung in this very real and unique way. Perfect voice in my book:)

Love Zooey's voice, nice surf guitar sound on this old R&B classic!

Omg wow. Is there anything Zooey Deschanel can't do? This is so raw and beautiful. And the original was by a man called SCREAMIN' Jay Hawkins, and I think he would be very pleased at this cover.

Good lord she's amazing!!!

SHE SO TALENTED

I knew she could sing but I didn't know she can SANNNG! I seriously didn't know she could hit those notes DUDE

People saying she's an "average singer" who's amazing then to you? They must truly be the best singer in the world because I wouldn't call this average at all.

Never knew she sang - outstanding and haunting version of this classic tune

I had no idea she had these pipes! Awesome.

i liked this version her voice is amazing

PERFECT PERFORMANCE

Wow I'm so blown away I literally couldn't keep my mouth closed! I didn't know Zooey was this good.

She is gorgeous and so is his guitars! Great cover of a really hep tune.

There's a lot singers wish they could sing this good Love her !!!

This is the best I have ever heard her sound.

Jesus Christ, that's how you effin sing.. I knew she could sing but wow that was incredible

Zooey puts a spell on me every time without fail,and I love it!

I'm obsessed with this song. She sings it beautifully.

This was my intro to She & Him (a while back), thank you, Conan.

I saw them perform this live in New Haven for a Christmas show - it was AMAZING!!

Love how Conan was legit impressed.

wow. she sounds so great. nice voice!

Wow! Ms. Deschanel's vocals on this number are crazy awesome!!!

i think if she ever grew her bangs out, the world would end

This performance always gives me goosebumps!

I think singing is her true calling. Good songwriter as well.

When you do a cover, you must own it! They have taken possession!

WOW!!!!!! Zooey is amazing. Not only is she a great singer, but a great actress.

I love these two!

She's got pipes. Love her...

Un-freaking believable! Ive been in love with her since I saw this live on Conan. I love his reaction when he comes over to thank them. I was thinking pretty much the same thing. WOW. Saw Casey Abrams perform this song last night on Idol and I had to watch this again.

Amazing performance! They nailed it!

Her voice is phenomenal and he can play

Amazing performance by She and Him, lovely Zooey!

SHE'S SOOOOO TALENTED!!!!!!!

How are they that jaw droppingly good?!

Yep. To be geeky and specific: M. Ward uses a Boss RC20XL Loop Station. That's also how he manages to play two parts at once right before the end.

How can someone have so much talent and beauty,its just not fair.

Gosh I love this woman!

You people with negative comments have no idea what soul music is.

DAMN!!! SHE'S INCREDIBLE

OMG, dude!!! This woman can REALLY sing!!! Plus she's extremely beautiful. Enough said.

Wow... I took it for granted that she was only a star on New Girl... reality check needed!!! She has the perfect voice for sensual songs with a lot of raw emotion... I like it :)

I like this live. I can't say that for many songs/singers.

She knocks that one out of the park.

I've been searching for this one! I saw it on tv live that nigh...I was like Conan! "WOW" that's how it's done! Gonna share this with my best friend! She sings too!

I LOVE THEM SOO MUCH!!!

She's beautiful 😍😍😍😍

Zoey is a 17.45 on the 1-10 scale. Insanely beautiful, great actress, great singer, phenomenal voice, absolutely stunning eyes and I could go on. The absolute total package!!

OMG IM BUYING THIS LP

You can call me at 10: 59 but not 11 cause that's my rule now

This could have been in Twin Peaks somewhere.

absolute perfection

Chills and goose bumps!!!!!

Unbeleiveable

PERFECT VOICE

Her voice is amazing!!

love this

She is perfect.

i love the way how she scream you can feel it in your bones

Amazing voice!!! Great guitar man M.ward!!!

oh my God! she sings amazingly great!

Omg. What a voice. Is this dream or something.

This is amazing!!

They are amazing !! Bravo !!

SHE IS AMAZING LIVE

Loved her in New Girl too,. Soulful singing.

I feel like she put a spell on me with her delivery of this song.

I love you both, whole wholeheartedly

Jesus! What a voice!

Somewhere in that great beyond, at a joint called Gabe's Place the late, great Screamin Jay Hawkins is smiling this day. Well done Miss Zooey!

I love she.

She and Him....Rock!

I love this version :D

G.i.L ♤♤♤~!~ she has one of the most beautiful voice of all time

I and the mic just melted.

Phenomenal !